期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 24, 页码 9196-9199出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja202012s
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资金
- NIGMS [P50 GM069721]
Introducing a silyl group at one of the internal olefin positions in diolefinic substrates results in E-selective olefin formation in macrocyclic ring-forming metathesis. The application of this method to a range of macrocyclic (E)-alkenylsiloxanes is described. Protodesilylation of alkenylsiloxane products yields novel Z-configured macrocycles.
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