期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 17, 页码 6517-6520出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja200712f
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资金
- National Institutes of Health [NIGMS R01 GM58133]
- National Science Foundation [CRIF 0840451]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0840451] Funding Source: National Science Foundation
The enantioselective crotylation of aldehydes with 1,2-diaminochlorocrotylsilane reagents is effectively catalyzed by Sc(OTf)(3). The one significant limitation on the utility of these reagents - substrate scope - has thus been addressed. The net result is the most comprehensive and highly practical method for enantioselective aldehyde crotylation yet advanced.
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