期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 27, 页码 10352-10355出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja202969z
关键词
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资金
- National Institute of General Medical Sciences, National Institutes of Health [GM-087620]
- National Science Foundation [CHE-0848982]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0848982] Funding Source: National Science Foundation
A highly efficient enantioselective C-H insertion of azavinyl carbenes into unactivated alkanes has been developed. These transition metal carbenes are directly generated from readily available and stable 1-sulfonyl-1,2,3-triazoles in the presence of chiral Rh(II) carboxylates and are used for C-H functionalization of alkanes to access a variety of beta-chiral sulfonamides.
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