期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 23, 页码 8877-8879出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja203227q
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资金
- National Science Foundation [CHE-0955864]
- Boehringer Ingelheim
- DuPont
- Eli Lilly
- University of California, Los Angeles
We report the total synthesis of (+/-)-aspidophylline A, one of many complex furoindoline-containing alkaloids that has not been synthesized previously. Our route features a number of key transformations, including a Heck cyclization to assemble the [3.3.1]-bicyclic scaffold as well as a late-stage interrupted Fischer indolization to install the furoindoline and construct the natural product's pentacyclic framework.
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