期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 29, 页码 11046-11049出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja203133h
关键词
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资金
- National Heart Lung and Blood Institute of the National Institutes of Health [HHSN268201000046C]
- National Science Foundation [DMR-0906815, DMR-1032267]
- Welch Foundation [A-0001]
- NIH [P30 DC004665]
Synthetic asymmetrical systems, Janus particles and patchy particles, are capable of undergoing hierarchical assembly processes that mimic those of Nature, to serve as switchable devices, optical probes, phase-transfer catalysts, and multifunctional drug carriers, each of which benefits from opposing surface patterns that behave differently. Production of nanometer-sized Janus particles that are equipped with efficient chemistries remains a challenge. A robust Janus-faced polymer nanoparticle framework that presents two orthogonally click-reactive surface chemistries has been generated by a recyclable strategy that involves reactive functional group transfer by templating against gold nanoparticle substrates. This anisotropic functionalization approach is compatible with a wide range of soft materials, providing Janus nanoparticles for the construction of dual-functionalized devices by accurately controlling chemical functionality at the nanoscopic level.
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