期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 133, 期 15, 页码 5692-5694出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja200210t
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资金
- National Science Foundation [DMR-0706559, CHE-0911543, CHE-0802907]
- DOE Basic Energy Sciences [BES-SC0002160]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [911543] Funding Source: National Science Foundation
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0802907] Funding Source: National Science Foundation
We demonstrate a modular click-based functionalization scheme that allows inexpensive conductive diamond samples to serve as an ultrastable platform for surface-tethered electrochemically active molecules stable out to similar to 1.3 V vs Ag/AgCl. We have cycled surface-tethered Ru(tpy)(2) to this potential more than 1 million times with little or no degradation in propylene carbonate and only slightly reduced stability in water and acetonitrile.
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