期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 132, 期 9, 页码 2856-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja909716k
关键词
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资金
- CAS
- NSFC [20821002, 20872155, 20972175]
- 973-program [2009CB825300]
- STCSM [08PJ1411600, 08dj1400100]
A novel palladium-catalyzed intermolecular aminofluorination of styrenes, with N-fluorobenzenesulfonimide (NFSI) functioning not only as a fluorinating reagent but also as an aminating reagent, has been developed. The reaction afforded vicinal fluoroamine products With very high regioselectivity. This transformation may involve fluoropalladation of styrene as a key step for C-F bond formation, The bidental nitrogen ligand is crucial to achieving the transformation successfully.
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