期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 132, 期 12, 页码 4092-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja1001407
关键词
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资金
- EPSRC
- University of Nottingham
- Royal Society Wolfson Merit Award
- ERC
- EU-FP6
- Engineering and Physical Sciences Research Council [EP/C528964/1] Funding Source: researchfish
Neutron powder diffraction experiments on D-2-loaded NOTT-112 reveal that the axial sites of exposed Cu(II) ions in the smallest cuboctahedral cages are the first, strongest binding sites for D-2 leading to an overall discrimination between the two types of exposed Cu(II) sites at the paddlewheel nodes. Thus, the Cu(II) centers within the cuboctahedral cage are the first sites of D-2 binding with a Cu-D-2 distance of 2.23(1) angstrom.
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