期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 132, 期 11, 页码 3680-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja1010866
关键词
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资金
- Scripps Research Institute
- National Institutes of Health [NIGMS, 1 R01 GM084019-01A1]
- Bristol Myers Squibb
- National Science Foundation
- Department of Defense
- Skagggs Oxford Scholarship
The first Pd(II)-catalyzed sp(3) C-H olefination reaction has been developed using N-arylamide directing groups. Following olefination, the resulting intermediates were found to undergo rapid 1,4-addition to give the corresponding gamma-lactams. Notably, this method was effective with substrates containing a-hydrogen atoms and could be applied to effect methylene C-H olefination of cyclopropane Substrates.
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