期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 132, 期 41, 页码 14418-14420出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja107328g
关键词
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资金
- NSF [CHE-0639094, CHE-0541745]
- NIH [RR027690]
- California Institute of Technology
- Baxter Foundation
(R)-BINOL center dot SnCl4 was found to catalyze a formal [3 + 2] cycloaddition reaction between C(3)-substituted indoles and 2-amidoacrylates to provide pyrroloindolines. A variety of pyrroloindolines were prepared with high enantioselectivity in one step from simple precursors. This methodology is expected to facilitate the total synthesis of pyrroloindoline alkaloids, an important class of biologically active natural products.
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