期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 8, 页码 2824-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja809372u
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资金
- DARPA [N00014-06-1-0897]
- Office of Naval Research [N00014-08-1-0928]
- AFOSR [FA9550-06-1-0192]
- National Science Foundation [DMR-0120967]
- NSF [ECS-0335765]
Combining a strong donor, tris(dodecyloxy)phenyl)-dithieno[3,2-b:2',3'-d]pyrrole, with a strong acceptor, 4,8-dithien-2-yl-2 lambda(4)delta(2)-benzo[1,2-c;4,5-c']bis[1,2,5]thiadiazole, has yielded the lowest bandgap, soluble, spray-processable polymer to date. The polymer has access to four different redox states and shows ambipolar behavior in OFETs. Multiple techniques, including transmission/absorption spectroscopy on SWCNTs and reflectance spectroscopy on gold were used to accurately estimate the optical bandgap at 0.5-0.6 eV, which correlates well to theoretical calculations.
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