期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 11, 页码 3796-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja8054595
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资金
- NIGMS NIH HHS [R01 GM073836-02S1, R01 GM073836-03, R01-GM073836, R01 GM073836] Funding Source: Medline
- PHS HHS [02S1] Funding Source: Medline
This communication describes the rational design and synthesis of the remarkably stable Pd-IV monoaryl fluoride complex (t-Bu-bpy)Pd-IV(p-FC6H4)(F)(2)(FHF) (t-Bu-bpy 4,4'-di-tert-butyl-2,2'-bipyridine). This and related complexes undergo Ar-F bond formation in the presence of F+ sources. This work serves as a foundation for the development of Pd-II/IV-catatyzed coupling reactions to form aryl fluorides.
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