期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 29, 页码 9900-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja903880q
关键词
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资金
- National Institutes of Health (NIH) [GM46059, F31M081905]
- Amgen,
- Boehringer-Ingelheim
- Merck
- Nippon Chemical
- BASF (Pd compounds
The enantioselective alpha-arylation and alpha-vinylation of oxindoles catalyzed by Pd and a biarylmonophosphine ligand with both axial and phosphorus-based chirogenicity is reported. The resultant quaternary carbon stereocenters are formed in high enantiomeric excess and the conditions tolerate a range of substitution on both the oxindole and the aryl/vinyl coupling partners.
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