期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 41, 页码 14626-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja906291n
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资金
- NSFC [20621091, 2067204, 0732002]
- Chang Jiang Scholars Program
The catalytic enantioselective synthesis of all-carbon quaternary stereogenic centers in spirocyclic diketones has been achieved for the first time by an unprecedented asymmetric vinylogous alpha-ketol rearrangement in which an enantiocontrotled semipinacol-type 1,2-carbon migration was realized using multifunctional cinchona-modified primary amine catalysis.
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