期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 9, 页码 3124-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja809897f
关键词
-
资金
- National Science Foundation [CHE-0619638]
An oxidative carbonylation reaction that generates acid chloride functionality has been developed. Furthermore, this aminochlorocarbonylation reaction has been merged with a catalytic Friedel-Crafts acylation to produce a highly efficient tandem multicatalytic synthesis of pyrrolidinyl ketones. Significant variation of the aromatic nucleophile and substrate are shown. Two examples of incorporation of this method in triple-catalytic sequences are also demonstrated.
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