期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 2, 页码 412-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja8066308
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资金
- University of Minnesota
- American Chemical Society Petroleum Research Fund
Carbon-carbon sigma-bond activation is a contemporary challenge for organometallic chemistry and catalysis. Herein, we disclose a new alkene carboacylation reaction initiated by quinoline-directed, rhodium-catalyzed C-C sigma bond activation. The alkene carboacylation allows for the construction of all-carbon quaternary centers, with a broad substrate scope, providing access to carbocyclic and heterocyclic ring systems in good to excellent yields.
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