期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 19, 页码 6678-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja9025243
关键词
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资金
- George Buchi Graduate Fellowship
Water is an effective promoter of the endo-selective opening of trisubstituted epoxides, enabling related cascades leading to a variety of substituted ladder polyether structures. When used in conjunction with a tetrahydropyran-templated nucleophile, water can overcome the powerful electronic directing effect of a methyl substituent at either site of the epoxide, making water a uniquely versatile medium and promoter of epoxide opening.
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