期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 11, 页码 3838-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja900023k
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资金
- Center for Chemical Innovation grant from the NSF [CHE-0533150]
- Chesonis Family Foundation
- Jane Coffin Childs Memorial Fund for Medicinal Research
- Department of Defense for a predoctoral fellowship (NDSEG)
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [0802907] Funding Source: National Science Foundation
A cobalt-phosphate water-oxidizing catalyst forms from the oxidation of Co2+ to Co3+ in the presence of phosphate. We have employed radioactive Co-57 and P-32 isotopes to probe the dynamics of this catalyst during water-oxidation catalysis. We show that the catalyst is self-heating and that phosphate is the crucial factor responsible for repair.
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