期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 37, 页码 13244-13245出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja9063487
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资金
- UC Berkeley, Eli Lilly, Johnson and Johnson, and AstraZeneca
- NSF
- Alfred P. Sloan Fellow
- Camille Dreyfus Teacher-Scholar
Total synthesis of the Galbulimima alkaloid G. B. 13 was achieved utilizing a functionalized pyridine moiety as a piperidine surrogate. Key to the success of the synthesis was the development of an unprecedented rhodium-catalyzed 1,2-addition of an arylboronic ester into an unactivated ketone.
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