期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 131, 期 51, 页码 18252-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja9088296
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资金
- National Science Council of the Republic of China [NSC-96-2113-M-007-020MY3]
A convenient and highly regioselective method for the synthesis of 5-methylenepyrrolidinone derivatives from various nitrites and acrylamides via a cobalt-catalyzed reductive coupling reaction is described. A possible mechanism that involves the formation of a cobaltaazacyclopentene intermediate from nitrite and acrylamide, protonation, keto-amide cyclization, and dehydration is proposed.
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