期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 130, 期 38, 页码 12590-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja804577q
关键词
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资金
- NSF
- NIH
Hydrophobic thiazolium and imidazolium coenzyme mimics in the presence of modified-polyethylenimine enzyme mimics catalyze the benzoin condensation 2300-3300 times faster than the coenzyme mimics alone. Polycationic enzyme mimics provide not only a hydrophobic binding domain for coenzyme and substrate, but also electrostatic stabilization of anionic species that arise along the reaction pathway of the benzoin condensation.
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