期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 130, 期 39, 页码 12846-+出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja802989v
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资金
- Schweizer Nationalfunds
- University of Zurich
The first visual fluorescence-based assay for the peroxide explosive triacetone triperoxide (TATP) is described. The assay is based on a conceptually new fluorescence signaling mechanism, in which nonemissive pyrenyl sulfoxide profluorophores are oxidized to visibly emissive pyrenyl sulfones. Although not without limitations, these first-generation fluorescent probes can provide a visual response to ca. 100 nmol of TATP. In addition, the success of this assay suggests the potential for broader application of aryl sulfoxides in fluorescent chemosensing.
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