期刊
JOURNAL OF POWER SOURCES
卷 260, 期 -, 页码 57-61出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2014.02.112
关键词
Stabilized Lithium Metal Powder; Prelithiation; Graphite anode; Solid electrolyte interface formation; Lithium-ion battery
资金
- Assistant Secretary for Energy Efficiency, Vehicle Technologies Office of the U.S. Department of Energy under the Industry-Laboratory Integrated Research Program (ILIRP)
- Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231]
Stabilized Lithium Metal Powder (SLMP (R)) was applied in graphite anode and the effects of this prelithiation method to cell performance were investigated. Performance of prelithiated cells was compared with that of regular graphite based cells. The first cycle capacity loss of SLMP prelithiated cell was largely reduced and the corresponding first cycle Coulombic efficiency was significantly improved. The graphite/NMC cell with SLMP prelithiation but without any standard cell formation process showed better cycle performance than that of none SLMP containing cell with standard formation process. Prelithiation of graphite electrode with SLMP promote stable solid electrolyte interface (SEI) formation on the surface of graphite anode. Application of SLMP in lithium-ion battery thus provides an effective method to enhance capacity, and promises a low cost SEI formation process. This also implies the potential use of other promising anode materials, such as Si and Sn that have large first cycle capacity loss, in commercial lithium-ion batteries. Published by Elsevier B.V.
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