期刊
JOURNAL OF POWER SOURCES
卷 196, 期 7, 页码 3683-3687出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.jpowsour.2010.12.063
关键词
Electrophoretic deposition (EPD); Titanium dioxide (TiO2); Dye-sensitized solar cells (DSCs); Low-temperature fabrication; Photovoltaics
资金
- National Science Council of Taiwan [NSC-99-2112-M-006-017-MY3, NSC-99-2221-E-009-095-MY3]
- Industrial Technology Research Institute [9301XS6A10]
- Bureau of Energy, Ministry of Economic Affairs [9455DI2110]
A multiple electrophoretic deposition (EPD) of binder-free TiO2 photoanode has been developed to successfully fill the crack occurring after air-drying on the first EPD-TiO2 film surface. With the slow 2nd EPD, high quality TiO2 thin films are acquired on flexible ITO/PEN substrates at room temperature and the device efficiency of the dye-sensitized solar cell achieved 5.54% with a high fill factor of 0.721. Electrochemical impedance spectroscopy measurements analyze the great enhancement of the photovoltaic performance through multiple EPD. The electron diffusion coefficient improved by about 1 order of magnitude in crack-less multiple-EPD TiO2 films. With the scattering layer, the device reveals a high conversion efficiency of up to 6.63% under AM 1.5 G one sun irradiation, having a short circuit current density, open circuit voltage, and filling factor of 12.06 mA cm(-2), 0.763 V and 0.72, respectively. Crown Copyright (C) 2010 Published by Elsevier B.V. All rights reserved.
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