期刊
JOURNAL OF PHYSICS D-APPLIED PHYSICS
卷 46, 期 36, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/0022-3727/46/36/365303
关键词
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资金
- Czech project of MEYS
- KONTAKT II [LH12150]
- EC [II-20100033]
- Japan society for promotion of science (JSPS)
- JSPS
- Ministry of Health Labour and Welfare
Luminescence processes in the undoped and Pr3+-doped (Gd,RE)(3)(Ga,Al)(5)O-12, RE = Lu,Y, multicomponent garnets are studied by time-resolved photoluminescence spectroscopy. Energy transfer processes between Pr3+ and Gd3+ causing significant deterioration of the scintillation performance are considered in detail. As is shown in current work, an overlap of the 5d(1)-H-3(4) emission transition of Pr3+ and S-8-P-6(x) absorption transition of Gd3+ results in unwanted depletion of Pr3+ 5d(1) excited state and is further intensified by the concentration quenching in the Gd3+-sublattice. This process explains a drastic decrease of light yield in Pr3+-doped Gd3+-containing multicomponent garnets observed in a previous work.
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