期刊
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS
卷 42, 期 12, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-4075/42/12/125101
关键词
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资金
- National Science Foundation [PHY-05-55699]
- Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences Division of the US Department of Energy [DE-AC03-76SF00098]
The fragmentation dynamics of core-excited methanoic acid (formic acid) has been studied by means of partial anion-and cation-yield measurements around the C K ionization threshold. All detectable ionic fragments are reported, and significant differences among partial-ion yields are observed. Possible dissociation pathways are discussed. We confirm experimentally the mixed A* molecular/3s Rydberg character of the resonance at 292.1 eV. Atomic rearrangements after photoabsorption leading to the formation of novel cationic fragments and selective fragmentation to the CH2O2+ ion are also reported.
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