期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 5, 期 8, 页码 1400-1411出版社
AMER CHEMICAL SOC
DOI: 10.1021/jz5004044
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- AIST
- METI
- JSPS
Metal-organic frameworks (MOFs) are highly ordered crystalline porous materials prepared by the self-assembly of metal ions and organic linkers having low-density framework structures of diversified topologies with tunable pore sizes and exceptionally large surface areas. Other than outstanding gas/molecule storage properties, loading of metal nanoparticles (MNPs) into the pores of MOFs could afford heterogeneous catalysts having advantages of controlling the particle growth to a nanosize region, resulting in highly active sites and enhanced catalytic performances, and these entrapped MNPs within MOF pores could be accessed by reactants for chemical transformations. This is a rapidly developing research area, and this Perspective addresses current achievements and future challenges for diverse MOF-immobilized MNPs within their pores, focusing especially on their preparation, characterization, and application as heterogeneous catalysts.
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