期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 1, 期 6, 页码 993-996出版社
AMER CHEMICAL SOC
DOI: 10.1021/jz100050y
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资金
- University of Warwick
- EPSRC [EP/E011187]
- University Research Fellowship
- EPSRC [EP/E011187/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/E011187/1] Funding Source: researchfish
Despite the extensive investigations thus far, there is still debate regarding the role of the repulsive pi sigma* state in the photochemistry of adenine. We present evidence that suggests that H-atom elimination via both the azole group (N-9) and the often overlooked amino group (N-6) occurs following excitation at 200 nm. In contrast, excitation at 266 nm supports the view that the role of the pi sigma* states is minimal.
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