期刊
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
卷 2, 期 1, 页码 25-33出版社
AMER CHEMICAL SOC
DOI: 10.1021/jz101550d
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类别
资金
- National Science Foundation
- American Chemical Society
- Kentucky Science and Engineering Foundation
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1012351] Funding Source: National Science Foundation
High-resolution electron spectroscopy combines pulsed ionization zero-electron kinetic energy (ZEKE) detection with in situ laser-assisted synthesis and supersonic expansion. The technique offers sub-meV spectral resolution for the electron spectra of metal complexes and is a powerful tool to study their bonding and structures. This Perspective presents recent progress in single-photon ZEKE spectroscopy of metal-aromatic complexes and on the determination of the electron spin multiplicities, metal binding sites and modes, rotational conformers, and conformational changes of these critical species in organometallic chemistry.
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