期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 117, 期 44, 页码 22805-22810出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp4069027
关键词
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资金
- Japan Society for the Promotion of Science (jSPS)
- Grants-in-Aid for Scientific Research [23360356, 11F01769] Funding Source: KAKEN
Palladium nanoparticles were immobilized within the pores of metal organic frameworks MIL-125 and amine-functionalized NH2-MIL-125 using photoassisted and ion exchange deposition methods. The resulting materials showed a very high activity for hydrogen production at ambient temperature in comparison to other titanium-based porous materials. The amine groups in NH2-MIL-125 greatly increased the H-2-generating activity and acted as a stabilizer of Pd NPs. The photoassisted deposition method was a more efficient method for producing highly dispersed small NPs in the MOF materials.
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