期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 117, 期 22, 页码 11850-11857出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp4027767
关键词
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资金
- KAKENHI [23310077, 24651143]
- Grants-in-Aid for Scientific Research [23310077, 24651143] Funding Source: KAKEN
We present a novel synthesis of ligand-free colloidal silicon nanocrystals (Si-NCs) that exhibits efficient photoluminescence (PL) in a wide energy range (0.85-1.8 eV) overcoming the bulk Si band gap limitation (1.12 eV). The key technology to achieve the wide-range controllable PL is the formation of donor and acceptor states in the band gap of Si-NCs by simultaneous doping of n- and p-type impurities. The colloidal Si-NCs are very stable in an ordinary laboratory atmosphere for more than a year. Furthermore, the PL spectra are very stable and are not at all affected even when the colloids are drop-cast on a substrate and dried in air. The engineering of the all-inorganic colloidal Si-NC and its optical data reported here are important steps for Si-based optoelectronic and biological applications.
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