期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 117, 期 17, 页码 8806-8812出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp4002059
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资金
- Natural Sciences and Engineering Research Council of Canada (NSERC)
- Canada Research Chair program
- NSERC
- National Research Council Canada
- Canadian Institutes of Health Research
- Province of Saskatchewan
- Western Economic Diversification Canada
- University of Saskatchewan
- Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]
- Deutsche Forschungsgemeinschaft (DFG) [SCHN 377/15-1]
- Fonds der Chemischen Industrie (FCI)
- Elite Network of Bavaria
- Nanosystems Initiative Munich
We have used a combination of X-ray and electron energy-loss spectroscopies along with DFT calculations to investigate the electronic structure of PTI/LiCl, a graphitic carbon nitride-type material with LiCl intercalation shown to photocatalyze the water-splitting reaction. The material is shown to have a band gap that is tunable with LiCl suggests that PTI/LiCl may be further optimized through loading, with a minimum gap of 2.2 eV when fully loaded. This control of their LiCl loading and shows that graphitic carbon nitride-type materials can be chemically tuned to improve their photocatalytic activity.
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