期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 116, 期 23, 页码 12468-12474出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp303120d
关键词
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资金
- A*STAR SERC [1021700144]
- Singapore MPA [MPA 23/04.15.03 RDP 009/10/102, MPA 23/04.15.03 RDP 020/10/113]
Novel CuxS/Cu (1 < x < 2) nanotubes were prepared by a facile wet chemical approach in polyethylene glycol (PEG). Here, Cu nanowires were presynthesized and then converted to nanotubes via a mass diffusion process. A thin PEG layer is physically adsorbed on the nanotube surface. The obtained CuxS/Cu nanotubes show good Li storage properties with stable cyclability upon Li ion insertion/extraction, which is attributed to the existence of the PEG capping and the reduced dissolution of Li polysulfides into the electrolytes. Furthermore, CuxS/Cu nanotubes with 10 wt % Cu show promising rate capabilities (a fifth-cycle discharge capacity of 282 mA h g(-1) at a current density of 5 A g(-1)) due to the enhanced kinetics of charge transfer.
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