期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 116, 期 46, 页码 24681-24689出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp308783y
关键词
-
资金
- EPSRC under the Hydrogen and Fuel Cells Supergen initiative
This paper presents in situ FTIR studies on the electrochemical oxidation of ethanol at polycrystalline Pt in 0.1 M KOH; the data obtained with C2H5OH are compared to results obtained using C2D5OD under the same conditions. The work continues our earlier studies on methanol and formate oxidation and supports the model formulated on the basis of these papers that, in contrast to acidic solution, under alkaline conditions intermediates are formed bonded through. 0 rather than C and that a number of mechanistic pathways are available differing very little in terms of activation energy.
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