期刊
JOURNAL OF PHYSICAL CHEMISTRY C
卷 115, 期 50, 页码 24494-24500出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp206485v
关键词
-
资金
- NSF [ECCS 0748091, CBET - 0930170, EECS - 0801774]
We report a simple scheme of anchoring crystalline ceria nanoparticles (CNPs) onto reduced graphene oxide (RGO) sheets. Two types of CNPs, consisting of predominantly either Ce3+ or Ce4+ valence states, were mixed with GO suspended in water, with simultaneous reduction using hydrazine to yield CNP/RGO composite. Structural and surface characterizations reveal a strong electrostatic interaction between the CNPs and the RGO. Electrical characterizations show that with increased oxygen vacancies from Ce4+ to Ce3+ states the predominantly ambipolar RGO transforms to n-type CNP/RGO composites due to the electrostatic interaction between the localized electrons in oxygen vacancy sites of CNPs and mobile holes in RGO.
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