期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 112, 期 29, 页码 6522-6526出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp800589j
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The excited state dynamics of Zn2+, Fe3+, and Mn3+ meso-tetra(sulfonatophenyl) porphyrin complexes were investigated with a Z-scan technique at 532 nm using 70 ps and 120 fs single pulses and 200 ns pulse trains of a Q-switched and mode locked laser. We determined the characteristic interconversion and intersystem crossing times, quantum yields of the excited S-1 state, and S-1 -> S-n and T-1 -> T-n transition cross-sections. The ground state cross-sections were obtained using UV-vis absorption spectroscopy, and a five-energy-level diagram was used to yield the photophysical parameters mentioned previously.
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