期刊
PHYSICAL REVIEW B
卷 92, 期 13, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.92.134412
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资金
- DST, India [SR/S2/RJN-76/2010, SB/S2/CMP-001/2013]
- UGC-CSIR India
We report the structure, magnetic, and thermal property measurements on single-crystalline and polycrystalline samples of the Ru-substituted honeycomb lattice iridate Na2Ir1-xRuxO3 (x = 0,0.05,0.1,0.15,0.2,0.3,0.5). The evolution of magnetism in Na2Ir1-xRuxO3 has been studied using dc and ac magnetic susceptibilities and heat-capacity measurements. The parent compound Na2IrO3 is a spin-orbit-driven Mott insulator with magnetic order of reduced moments below T-N = 15 K. In the Ru-substituted samples the antiferromagnetic long-range state is replaced by a spin-glass-like state even for the smallest substitution suggesting that the magnetic order in Na2IrO3 is extremely fragile. We argue that these behaviors indicate the importance of nearest-neighbor magnetic exchange in the parent Na2IrO3. Additionally, all samples show insulating electrical transport.
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