期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 79, 期 3, 页码 1377-1385出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo4027885
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资金
- MEXT, Japan
- JSPS, Japan
- Grants-in-Aid for Scientific Research [25620084] Funding Source: KAKEN
A manganese-mediated dehydrogenative direct alkylation of 2-pyridones with diethyl malonates has been developed. A similar reaction system is applicable to the direct arylation with arylboronic acids. These manganese-based reactions occur regioselectively at the C3 position of the 2-pyridones. The observed high C3 regioselectivity can complement precedented C-H functionalization protocols of the 2-pyridones in view of the site selectivity.
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