期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 77, 期 5, 页码 2310-2330出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo202558f
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资金
- Deutsche Forschungsgemeinschaft
- Bayer-Schering Pharma AG
- Chemtura Organometallics GmbH Bergkamen
- Bayer Services GmbH
- BASF AG
- Sasol GmbH
Extensive studies of asymmetric cross-aldol addition between enolizable aldehydes are described and provide a deeper insight into histidine-catalyzed aldol additions. In particular, aspects of enantio- as well as diastereoselectivity of these reactions are discussed. Rules and predictions of configurative outcome are explained by using different transition-state models. These discussions are confirmed by extensive computations.
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