期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 76, 期 10, 页码 3644-3653出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo200359c
关键词
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资金
- National Science Foundation [CHE-0911212]
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [0911212] Funding Source: National Science Foundation
Processes that form multiple carbon-carbon bonds in one operation can generate molecular complexity quickly and therefore be used to shorten syntheses of desirable molecules. We selected the hetero-Pauson-Khand (HPK) cycloaddition and ring-closing metathesis (RCM) as two unique carbon-carbon bond-forming reactions that could be united in a tandem ruthenium-catalyzed process. In doing so, complex polycyclic products can be obtained in one reaction vessel from acyclic precursors using a single ruthenium additive that can catalyze sequentially two mechanistically distinct transformations.
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