期刊
PHYSICAL REVIEW A
卷 91, 期 1, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevA.91.013406
关键词
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资金
- German Research Foundation (DFG) [RU 420/7-1]
- U.S. National Science Foundation
- Office of Science of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231, DE-AC05-00OR22725]
Photoionization of neutral atomic sulfur in the ground and metastable states was studied experimentally at a photon energy resolution of 44 meV (full width at half maximum). Relative cross section measurements were recorded by using tunable vacuum ultraviolet radiation in the energy range 9-30 eV obtained from a laser-produced plasma and the atomic species were generated by photolysis of molecular precursors. Photoionization of this atom is characterized by multiple Rydberg series of autoionizing resonances superimposed on a direct photoionization continuum. A wealth of resonance features observed in the experimental spectra are spectroscopically assigned and their energies and quantum defects tabulated. The cross section measurements are comparedwith state-of-the-art theoretical cross section calculations obtained from the Dirac Coulomb R-matrix method. Resonance series in the spectra are identified and compared, indicating similar features in both the theoretical and experimental spectra.
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