期刊
JOURNAL OF ORGANIC CHEMISTRY
卷 74, 期 21, 页码 8359-8368出版社
AMER CHEMICAL SOC
DOI: 10.1021/jo901986v
关键词
-
资金
- Ministerio de Ciencia c Innovacion, Spain [CTQ2006-00500/BQU]
- University of Barcelona
An indole-templated ring-closing metathesis or it 2-indolylacyl radical cyclization constitute the central steps of two alternative approaches developed to assemble the tricyclic ABC substructure of the indole alkaloid apparicine From this key intermediate, an intramolecular vinyl halide Heck reaction accomplished the closure of the strained 1-azabicyclo[4.2.2]decane framework of the alkaloid with concomitant incorporation of the exocyclic alkylidene substituents.
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