期刊
JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS
卷 29, 期 20, 页码 17591-17601出版社
SPRINGER
DOI: 10.1007/s10854-018-9862-x
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资金
- National Natural Science Foundation of China [21571160]
- National Natural Science Foundation of China-Henan Talents Fostering Joint Funds [U1504311]
- Key Research Projects of the Science and Technology Department of Henan Province [172102210544, 182102210153, 182102210619]
- Fundamental Research Funds for the Provincial Universities [18KYYWF0109]
- Doctoral Scientific Research Foundation of Zhengzhou University of Light Industry [2015BSJJ044]
g-C3N4/NH2-MIL-101(Fe) composites are successfully fabricated by a facile in situ solvothermal method. The as-prepared samples have been characterized by XRD, FTIR, XPS, FESEM, TEM, DRS and PL analysis. Under visible light irradiation, the g-C3N4/NH2-MIL-101(Fe) composite shows higher photocatalytic activities than bare g-C3N4 and NH2-MIL-101(Fe) for Cr(VI) reduction and MO degradation. The improved photocatalytic performances are ascribed to the efficient charge separation and transfer on the interface between g-C3N4 and NH2-MIL-101(Fe). Control experiments show that the pH value is vital for Cr(VI) reduction, and meanwhile, the addition of hole scavengers promotes the photocatalytic reduction significantly. Finally, a possible reaction mechanism had also been investigated in detail.
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