期刊
PARTICLE & PARTICLE SYSTEMS CHARACTERIZATION
卷 32, 期 11, 页码 1006-1011出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ppsc.201500095
关键词
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资金
- National High Technology Research and Development Program of China (863 Program) [2013AA050905]
- National Natural Science Foundation of China [21275151, 21271180]
- State Key Laboratory of Electroanalytical Chemistry [SKLEAC201302]
- Youth Innovation Promotion Association of CAS [2014188]
- Qingdao Key Lab of Solar Energy Utilization & Energy Storage Technology
Niobium nitride/nitrogen-doped graphene nanosheet hybrid materials are prepared by a simple hydrothermal method combined with ammonia annealing and their electrochemical performance is reported. It is found by scanning electron microscopy (SEM) and transmission electron microscopy (TEM) that the as-obtained niobium nitride nanoparticles are about 10-15 nm in size and homogeneously anchored on graphene. A non-aqueous lithium-ion capacitor is fabricated with an optimized mass loading of activated carbon cathode and the niobium nitride/nitrogen-doped graphene nanosheet anode, which delivers high energy densities of 122.7-98.4 W h kg(-1) at power densities of 100-2000 W kg(-1), respectively. The capacity retention is 81.7% after 1000 cycles at a current density of 500 mA g(-1). The high energy and power of this hybrid capacitor bridges the gap between conventional high specific energy lithium-ion batteries and high specific power electrochemical capacitors, which holds great potential applications in energy storage for hybrid electric vehicles.
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