期刊
JOURNAL OF INDUSTRIAL AND ENGINEERING CHEMISTRY
卷 19, 期 6, 页码 1968-1972出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.jiec.2013.03.005
关键词
Carbon; Lithium; Sulfur; Battery; Electrochemistry
资金
- Div Of Chem, Bioeng, Env, & Transp Sys
- Directorate For Engineering [1233250] Funding Source: National Science Foundation
The effect of carbon surface area on capacity is investigated in cathodes for lithium sulfur batteries. Carbon additives help overcome the low electrical conductivity of sulfur. Cathodes were prepared at 30 wt% sulfur on different activated carbons having unloaded BET surface areas of 1200-3200 m(2)/g. Sulfur utilization ranged from 33% to 83% of the theoretical capacity (1672 mAh/g) with a strong correlation to the accessible pore volumes having pore widths between 1 and 5 nm. Additionally, cathodes prepared at 12.5-68 wt% on an activated carbon having unloaded BET surface area of 3200 m(2)/g showed excessive sulfur loading provided little additional capacity. (C) 2013 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
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