期刊
ORGANIC PROCESS RESEARCH & DEVELOPMENT
卷 19, 期 7, 页码 872-877出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.oprd.5b00132
关键词
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资金
- National Center for Research and Development (NCBiR)
The ammonium tagged Hoveyda-type catalyst bearing sterically enlarged N-heterocyclic carbene ligand was synthesized and supported on SBA-15. The obtained heterogeneous olefin metathesis catalyst forms unprecedentedly stable Ru-methylidenes and provides products of ring-closing and cross metathesis with turnover numbers (TONs) up to 35 000 and turnover frequencies (TOFs) up to 1590 min(-1). The catalyst proved to be truly recyclable and effective in a continuous flow mode.
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