期刊
ORGANIC LETTERS
卷 17, 期 21, 页码 5404-5407出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b02728
关键词
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资金
- 1000-Youth Talents Plan
- Sun Yat-sen University
- National Natural Science Foundation of China [81402794, 21472250]
Cp*Co(III)-catalyzed annulations of 2-alkenylphenols with CO for the synthesis of coumarin derivatives have been developed. The reaction features mild reaction conditions, broad substrate scope, and good functional group tolerance. Preliminary mechanistic studies were conducted, suggesting that C-H activation is the turnover limiting step. Furthermore, the efficiency of this reaction was demonstrated by the rapid total synthesis of three natural products herniarin, xanthyletin, and seselin.
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