期刊
ORGANIC LETTERS
卷 17, 期 20, 页码 4940-4943出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b01932
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资金
- NRW Graduate School of Chemistry
- [SFB858]
Efficient construction of complex cylcopentane- or cyclohexane-fused delta-lactones employing redox activation of enals using a chiral N-heterocyclic carbene and LiCl as cooperative catalysts is described. The organocascade proceeds with excellent diastereo- (>99:1) and enantioselectivity (up to >99% cc) and comprises the formation of three bonds with three contiguous stereocenters.
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