期刊
ORGANIC LETTERS
卷 17, 期 17, 页码 4125-4127出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b02025
关键词
-
资金
- National Science Foundation of China [21402188]
A new way of forming the aza-o-xylylene with easily accessible 1,2-dihydroquinolines as precursor has been developed. The presence of an electron-donating group at the proper position of 1,2-clihydroquinoline was crucial for protonation of the alkene through dearomatization with a simple Bremsted acid. The in situ forming reactive intermediate was trapped with Hantzsch ester to afford tetrahydroquinolines in excellent yield and enantioselectivity.
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