期刊
ORGANIC LETTERS
卷 17, 期 21, 页码 5368-5371出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b02705
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资金
- National Science Council of Taiwan
- Centre for bioinformatics research of aiming for the Top University Plan of the National Chiao Tung University
- Ministry of Education, Taiwan
A mechanistic study of three-component reactions of various aromatic amines with a number of aldehydes and 1,3-diones was achieved. The unprecedented reaction involved a nucleophilic attack of an aromatic amine on the in situ generated Michael adduct intermediate followed by six-electron ring cyclizations. It is contrary to the common belief that advocates involvement of coupling reactions between a Knoevenagel adduct and an aromatic amine to deliver substituted tetrahydroacridinones.
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